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Study of the interlayer adhesion and warping during material extrusion-based additive manufacturing of a carbon nanotube/biobased thermoplastic polyurethane nanocomposite
dc.contributor.author | Candal, María Virginia | |
dc.contributor.author | Calafel Martínez, Miren Itxaso | |
dc.contributor.author | Fernández San Martín, Mercedes | |
dc.contributor.author | Aramburu Ocáriz, Nora | |
dc.contributor.author | Hernández Aguirresarobe, Roberto | |
dc.contributor.author | Guerrica Echevarría Estanga, Gonzalo María | |
dc.contributor.author | Santamaría Ibarburu, Pedro Antonio | |
dc.contributor.author | Müller Sánchez, Alejandro Jesús | |
dc.date.accessioned | 2021-04-26T18:17:00Z | |
dc.date.available | 2021-04-26T18:17:00Z | |
dc.date.issued | 2021-04-07 | |
dc.identifier.citation | Polymer 224 : (2021) Article ID 123734 | es_ES |
dc.identifier.issn | 0032-3861 | |
dc.identifier.uri | http://hdl.handle.net/10810/51192 | |
dc.description | Sustituido preprint por postprint 03-05-2023 | es_ES |
dc.description.abstract | A thermoplastic bio-polyurethane from renewable sources (TPU) and the nanocomposite developed by mixing it with carbon nanotubes (CNT) are investigated as potentially adequate for Material Extrusion-based Additive Manufacturing (EAM). Thermal and rheological features are studied from the perspective of their liaisons with printing adequacy and conditions. As predicted by rheology, both samples show good performance in filament elaboration and flow in the nozzle. Warpage is observed for TPU, but not for the nanocomposite, which is due to the effect of CNT nanoparticles on polymer chains dynamics. At the studied printing velocities, interlayer adhesion strength is independent of printing velocity implying that there is no significant chain orientation which can induce changes in the TPU entanglements. The nanocomposite shows a lower welding strength, notwithstanding both have the same chain entanglements density. This is explained by considering that the higher viscosity of TPU/CNT, as compared to TPU, reduces the melt diffusion coefficient. | es_ES |
dc.description.sponsorship | We would like to thank the financial support provided by the BIODEST project. This project has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 778092. This work has also received funding from MINECO through project MAT2017-83014-C2-1-P and from the Basque Government through grant IT1309-19. | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Elsevier | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/H2020/778092 | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO/MAT2017-83014-C2-1-P | es_ES |
dc.rights | info:eu-repo/semantics/openAccess | es_ES |
dc.subject | thermoplastic polyurethane | es_ES |
dc.subject | biobased TPU | es_ES |
dc.subject | carbon nanotubes | es_ES |
dc.subject | material extrusion-based additive | es_ES |
dc.subject | manufacturing | es_ES |
dc.subject | entanglements | es_ES |
dc.subject | inter-diffusion | es_ES |
dc.title | Study of the interlayer adhesion and warping during material extrusion-based additive manufacturing of a carbon nanotube/biobased thermoplastic polyurethane nanocomposite | es_ES |
dc.type | info:eu-repo/semantics/article | es_ES |
dc.rights.holder | © 2021 Elsevier Ltd under CC BY-NC-ND license (http://creativecommons.org/licenses/by- nc-nd/4.0/) | es_ES |
dc.relation.publisherversion | https://www.sciencedirect.com/science/article/pii/S0032386121003578?via%3Dihub | es_ES |
dc.identifier.doi | 10.1016/j.polymer.2021.123734 | |
dc.contributor.funder | European Commission | |
dc.departamentoes | Ciencia y tecnología de polímeros | es_ES |
dc.departamentoeu | Polimeroen zientzia eta teknologia | es_ES |